So if Alistar's W is becoming a skillshot can you finally let him jungle again?

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Big manly shield man is a support. Big manly cow (not really a) man being a support isn't farfetched.

The problem with Alistar virtually anywhere else is his somewhat overbearing lack of counter play.

Yes but Braum is all about helping people with his muscles, very different from Cowman

Alistar is all about beating the ever living shit out of people, which fits more with something like Renekton